Toward atomic resolution diffractive imaging of isolated molecules with x-ray free-electron lasers
2014-03-11 | journal article
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Toward atomic resolution diffractive imaging of isolated molecules with x-ray free-electron lasers
Stern, S.; Holmegaard, L.; Filsinger, F.; Rouzée, A.; Rudenko, A.; Johnsson, P. & Martin, A. V. et al. (2014)
Faraday Discussions, 171 pp. 393-418. DOI: https://doi.org/10.1039/C4FD00028E
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Details
- Authors
- Stern, Stephan; Holmegaard, Lotte; Filsinger, Frank; Rouzée, Arnaud; Rudenko, Artem; Johnsson, Per; Martin, Andrew V.; Barty, Anton; Bostedt, Christoph; Bozek, John D.; Coffee, Ryan N.; Epp, Sascha; Erk, Benjamin; Foucar, Lutz; Hartmann, Robert; Kimmel, Nils; Kühnel, Kai-Uwe; Maurer, Jochen; Messerschmidt, Marc; Rudek, Benedikt; Starodub, Dmitri G.; Thøgersen, Jan; Weidenspointner, Georg; White, Thomas A.; Stapelfeldt, Henrik; Rolles, Daniel; Chapman, Henry N.; Küpper, Jochen
- Abstract
- We give a detailed account of the theoretical analysis and the experimental results of an x-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i. e., picometers and femtoseconds, using x-ray free-electron lasers.
- Issue Date
- 11-March-2014
- Journal
- Faraday Discussions
- Working Group
- RG Techert (Structural Dynamics in Chemical Systems)
- ISSN
- 1359-6640; 1364-5498
